Substitution versus Elimination

Substitution versus Elimination: MDCAT Chemistry notes

Substitution versus Elimination for MDCAT: SN1, SN2, E1 and E2 mechanisms, carbocations, molecularity and order, aqueous vs alcoholic KOH and products.

Unit: Alkyl Halides · Updated

Two competing reactions

A nucleophile such as $\mathrm{OH^-}$ or $\mathrm{C_2H_5O^-}$ is also a base. When it meets an alkyl halide it can either attack the $\alpha$-carbon and replace the halogen (substitution) or remove a proton from the $\beta$-carbon so that HX is lost and a C=C forms (elimination, dehydrohalogenation). Both reactions need the halide to leave, so a better leaving group ($\mathrm{I^- > Br^- > Cl^-}$) speeds up both in the same way. SN2 competes with E2, and SN1 competes with E1.

SN2 mechanism

  • One step, concerted: the nucleophile attacks from the back side while the C–X bond breaks, through a single transition state (no intermediate).
  • Rate = $k[\mathrm{RX}][\mathrm{Nu^-}]$: second order, bimolecular (molecularity 2).
  • Gives inversion of configuration.
  • Favoured by primary halides, which are least crowded. Primary halides react almost always by SN2.

SN1 mechanism

  • Two steps: (1) the C–X bond breaks slowly to give a carbocation intermediate; (2) the nucleophile attacks the carbocation quickly.
  • Rate = $k[\mathrm{RX}]$: first order, unimolecular (molecularity 1).
  • The carbocation is sp$^2$, planar, with an empty p-orbital. The nucleophile can attack either face, so a chiral substrate gives a racemic mixture.
  • Reactivity tertiary > secondary > primary, because the tertiary carbocation is most stable.

E2 and E1

E2 is a one-step, bimolecular elimination in which a strong base removes a $\beta$-hydrogen as the halide leaves. E1 is two-step and goes through the same carbocation as SN1, which then loses a proton. In both, the product is an alkene.

FeatureSN1SN2E1E2
Steps2121
Order / molecularity1 / 12 / 21 / 12 / 2
IntermediateCarbocationNone (transition state)CarbocationNone
Best substrate3$^\circ$1$^\circ$3$^\circ$3$^\circ$, 2$^\circ$ with strong base
ProductSubstitutionSubstitutionAlkeneAlkene

What decides the winner

ConditionFavours
Aqueous KOH/NaOH, lower temperatureSubstitution → alcohol
Alcoholic KOH, heatElimination → alkene
Strong, bulky base (e.g. ethoxide with a 2$^\circ$/3$^\circ$ halide)Elimination
Higher temperatureElimination
Less polar solvent (alcohol rather than water)Elimination

Examples:

  • 1-chlorobutane + aqueous NaOH → 1-butanol.
  • 2-bromobutane + alcoholic KOH → 2-butene (major, the more substituted alkene).
  • 2-bromopropane (or 1-bromopropane) with alcoholic KOH or sodium ethoxide → propene as the major product.

Common MDCAT traps

  • "Bond breaking and bond forming at the same time" is SN2, not SN1 or E1.
  • SN1 is two-step, first order, molecularity 1; SN2 is one-step, second order, molecularity 2.
  • Strong bases and high temperature favour elimination, not substitution.
  • Aqueous KOH gives alcohol; alcoholic KOH gives alkene. Zn dust and conc. $\mathrm{H_2SO_4}$ are not used for dehydrohalogenation.
  • The SN1 intermediate is a carbocation, not a carbanion or free radical.

Quick revision

  • SN1 order: 3$^\circ$ > 2$^\circ$ > 1$^\circ$; SN2 order: 1$^\circ$ > 2$^\circ$ > 3$^\circ$.
  • Racemization in SN1 comes from the planar carbocation's empty p-orbital.
  • Leaving group plays the same role in substitution and elimination.
  • Elimination of HX from an alkyl halide gives an alkene.

Test yourself

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